This is the Proceedings of the Taniguchi International Symposium on "Relaxation of Elementary Excitations" which was held October 12-16,1979, at Susono-shi (at the foot of f1t. Fuji) in Japan. The pleasant atmosphere of the Symposium is evidenced in the picture of the participants shown on the next page. The purpose of the symposium was to provide an opportunity for a limited number of active researchers to meet and to discuss relaxation processes and related phenomena not only of excitons and phonons in solids but also electronic and vibrational excitations in molecules and biological systems. First, the lattice relaxation, i.e., multi-phonon process, associated with electronic excitation, which plays important roles in self-trapping of an exciton and a particle (electron and hole) and also in degradation of semi­ conductor lasers, is discussed. Second, this lattice relaxation is studied as the intermediate state interaction in the second-order optical responses, i.e., in connection with the competitive behavior of Raman scattering and luminescence. Third, relaxation mechanisms and relaxation constants are by spectroscopic methods as well as by genuine nonlinear optical determined phenomena. Conversely the relaxation is decisive in coherent nonlinear optical phenomena such as laser, superradiance, and optical bistability. Fourth, the role played by relaxation processes is discussed for optical phenomena in macromolecules and biological system such as photosynthesis.

Inhalt

I. Lattice Relaxation.- Electrons, Holes and Excitons in Deformable Lattice.- Large Lattice Relaxation Processes in Semiconductors.- Nonradiative Transition During Lattice Relaxation in Localized Electron-Phonon System.- II. Intermediate State Interaction.- Resonant Raman Scattering and Luminescence.- First and Second Order Optical Responses in Exciton-Phonon System.- Vibronic Spectra of Molecular Crystals: Dynamic Theory and Comparison with Experiment.- Ultrafast Vibrational Relaxation Processes of Polyatomic Molecules, Investigated by Picosecond Light Pulses.- III. Nonlinear Optical Phenomena.- Relaxation Study in the Extremely Short Time Region by Stationary and Transient Nonlinear Optical Spectroscopy.- Thermodynamics and Transient Dynamics of Simple Optical Systems with Instability.- New Photon-Echo Phenomena in a Localized-Electron Phonon System.- IV. Molecular Crystal and Biological System.- Relaxation of Electronic Excitation in Biology: The Initial Processing of Photon Energy and Information.- The Origin of the J Band.- V. Molecular System.- Infrared Laser Chemistry.- Multiphoton Vibrational Pumping of Optically Prepared NO2 Molecules.- An Experimental Study on Unimolecular Reactions Induced by Infrared Multiple Photon Absorption.- Theory of Collisionless Molecular Multiphoton Processes.- Unified Theory of Collisional Redistribution in Near-Resonance Light Scattering.- Energetics of the Photodissociation of Polyatomic Molecules.- Determination of Molecular Relaxation Constants by Coherent Transient Spectroscopy.- Index of Contributors.